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There were some changes made during the Activas acquisition in 2015, a lot of people started complaining that Armour wasn't as effective. I think the other major factor was that people were seeing a lot of huge price hikes, which might be why you're seeing some switching take place. I've heard good things with Naturethroid, but have never used it. After the Armour deal, it's been either compounded NDT through Defy or Cytomel through my GP on this end.

Also, if you're hitting 4.0pg/ml (2.0-4.4?) on 1 grain, that's pretty good. 1 grain will put me around 50% of reference range, 1.5 grains about 60%, which for me is fine, anything more gets me a little more jittery than desired. 4.0pg/ml on that same ref scale is 83%. Just be sure to compare how that sits in relation to your Free T4, and in relation to Reverse T3 with factoring the ratio, FT3/RT3.